Chirped pulse amplification

Chirped pulse amplification (CPA) is a technique for amplifying an ultrashort laser pulse up to the petawatt level, with the laser pulse being stretched out temporally and spectrally, then amplified, and then compressed again.^[1] The stretching and compression uses devices that ensure that the different color components of the pulse travel different distances.

CPA for lasers was introduced by Donna Strickland and Gérard Mourou at the University of Rochester in the mid-1980s,^[2] work for which they received the Nobel Prize in Physics in 2018.^[3]

CPA is the technique used by most high-powered lasers in the world.

Background

Before the introduction of CPA in the mid-1980s, the peak power of laser pulses was limited because a laser pulse at intensities of gigawatts per square centimeter causes serious damage to the gain medium through nonlinear processes such as self-focusing. For example, some of the most powerful compressed CPA laser beams, even in an unfocused large aperture (after exiting the compression grating) can exceed intensities of 700 GW/cm², which if allowed to propagate in air or the laser gain medium would instantly self-focus and form a plasma or cause filament propagation, both of which would ruin the original beam's desirable qualities and could even cause back-reflection potentially damaging the laser's components. In order to keep the intensity of laser pulses below the threshold of the nonlinear effects, the laser systems had to be large and expensive, and the peak power of laser pulses was limited to the high gigawatt level or terawatt level for very large multi-beam facilities.

In CPA, on the other hand, an ultrashort laser pulse is stretched out in time prior to introducing it to the gain medium using a pair of gratings that are arranged so that the low-frequency component of the laser pulse travels a shorter path than the high-frequency component does. After going through the grating pair, the laser pulse becomes positively chirped, that is, the high-frequency component lags behind the low-frequency component, and has longer pulse duration than the original by a factor of 1000 to 100000.

Then the stretched pulse, whose intensity is sufficiently low compared with the intensity limit of gigawatts per square centimeter, is safely introduced to the gain medium and amplified by a factor of a million or more. Finally, the amplified laser pulse is recompressed back to the original pulse width through reversal of the process of stretching, achieving orders-of-magnitude higher peak power than laser systems could generate before the invention of CPA.

In addition to the higher peak power, CPA makes it possible to miniaturize laser systems (the compressor being the biggest part). A compact high-power laser, known as a tabletop terawatt laser (T³ laser, typically delivering 1 joule of energy within 1 picosecond), can be created based on the CPA technique.^[4]

Stretcher and compressor design

There are several ways to construct compressors and stretchers. However, a typical Ti:sapphire-based chirped-pulse amplifier requires that the pulses are stretched to several hundred picoseconds, which means that the different wavelength components must experience about 10 cm difference in path length. The most practical way to achieve this is with grating-based stretchers and compressors. Stretchers and compressors are characterized by their dispersion. With negative dispersion, light with higher frequencies (shorter wavelengths) takes less time to travel through the device than light with lower frequencies (longer wavelengths). With positive dispersion, it is the other way around. In a CPA, the dispersions of the stretcher and compressor must cancel out. Because of practical considerations, the (high-power) compressor is usually designed with negative dispersion, and the (low-power) stretcher is therefore designed with positive dispersion.

In principle, the dispersion of an optical device is a function ${\displaystyle \tau (\omega )}$, where ${\displaystyle \tau }$ is the time delay experienced by a frequency component ${\displaystyle \omega }$. (Sometimes the phase ${\displaystyle \phi (\omega )=2\pi \tau (\omega )c/\lambda (\omega )}$ is used, where c is the speed of light and ${\displaystyle \lambda }$ is the wavelength.) Each component in the whole chain from the seed laser to the output of the compressor contributes to the dispersion. It turns out to be hard to tune the dispersions of the stretcher and compressor such that the resulting pulses are shorter than about 100 femtoseconds. For this, additional dispersive elements may be needed.

With gratings

Figure 1 shows the simplest grating configuration, where long-wavelength components travel a larger distance than the short-wavelength components (negative dispersion). Often, only a single grating is used, with extra mirrors such that the beam hits the grating four times rather than two times as shown in the picture.

Figure 1. Schematic layout of a grating-based compressor with ne­gative dispersion, i.e., the short wavelengths (in blue) come out first.

Figure 2. Dispersion orders of a grating compressor. (p = 2 − GDD, p = 3 − TOD, p = 4 − FOD, p = 5 − FiOD, p = 6 − SiOD, p = 7 − SeOD, p = 8 − EOD, p = 9 − NOD, p = 10 − TeOD)

This setup is normally used as a compressor since it does not involve transmissive components that could lead to unwanted side-effects when dealing with high-intensity pulses. The dispersion can be tuned easily by changing the distance between the two gratings. The introduced dispersion by such a compressor is often described in dispersion orders: the group delay dispersion (GGD), third order of dispersion (TOD) etc. Figure 2 shows the dispersion orders for a grating compressor with a groove density of ${\displaystyle \sigma =1700\;\mathrm {lines/mm} }$, an incidence angle of ${\displaystyle \theta _{in}=65^{\circ }}$, and a normal grating separation of ${\displaystyle L=25\;\mathrm {cm} }$, as described in the original design by Donna Strickland and Gérard Mourou (1985),^[2] and evaluated using Lah-Laguerre optical formalism - a generalized formulation of the high orders of dispersion.^[5][6]

Figure 3. Schematic layout of a grating-based stretcher. In this case, ${\displaystyle L<f}$, which leads to a positive dispersion, i.e. the long wavelengths (in red) come first.

Figure 3 shows a more complicated grating configuration that involves focusing elements, here depicted as lenses. The lenses are placed at a distance ${\displaystyle 2f}$ from each other (they act as a 1:1 telescope), and at a distance ${\displaystyle L}$ from the gratings. If ${\displaystyle L<f}$, the setup acts as a positive-dispersion stretcher and if ${\displaystyle L>f}$, it is a negative-dispersion stretcher. The ${\displaystyle L=f}$ case is used in Femtosecond pulse shaping. Usually, the focusing element is a spherical or cylindrical mirror rather than a lens. As with the configuration in Figure 1, it is possible to use an additional mirror and use a single grating rather than two separate ones. This setup requires that the beam diameter is very small compared to the length of the telescope; otherwise undesirable aberrations will be introduced. For this reason, it is normally used as a stretcher before the amplification stage, since the low-intensity seed pulses can be collimated to a beam with a small diameter.

With prisms

Main article: Prism compressor

Figure 4. Prism stretcher. This configuration has a positive dispersion. Although the different wavelengths appear to travel along very different paths, the effective path length differences are rather small, as indicated by the colors of the dispersed pulse.

Figure 5. Dispersion orders of a fused silica prism-pair compressor at 780 nm. (p = 2 − GDD, p = 3 − TOD, p = 4 − FOD, p = 5 − FiOD, p = 6 − SiOD, p = 7 − SeOD, p = 8 − EOD, p = 9 − NOD, p = 10 − TeOD)

It is possible to use prisms rather than gratings as dispersive elements, as in Figure 4. Despite such a simple change, the set-up behaves quite differently, as to first order no group delay dispersion is introduced. Such a stretcher/compressor can have both a positive or negative dispersion, depending on the geometry and the material properties of the prisms. With lenses, the sign of the dispersion can be reversed, similar to Figure 3. For a given distance between the dispersive elements, prisms generate much less dispersion than gratings. Prisms and gratings are sometimes combined to correct higher order dispersion ("grisms"), in which case the distance between the prisms is on the order of 10 meters rather than 50 cm as with a grating compressor. Gratings lose power into the other orders, while prisms lose power due to Rayleigh scattering. As an example, the dispersion orders of a fused silica prism-pair compressor are illustrated in Figure 5 for variable insertion depth of the first prism ${\displaystyle \ell _{1}}$. The dispersion is evaluated for laser pulses at ${\displaystyle 780{\text{ nm}}}$ with spectral bandwidth of ${\displaystyle \Delta \lambda =30{\text{ nm}}}$, using Lah-Laguerre optical formalism - a generalized formulation of the high orders of dispersion.^[5][6] The compressor parameters at near Brewster incidence angle are: normal distance between the prisms of ${\displaystyle L=30{\text{ cm}}}$, insertion depth of the second prism ${\displaystyle \ell _{2}={\text{1 mm}}}$ at ${\displaystyle \lambda _{min}}$ and an apex angle of the fused silica prisms ${\displaystyle \alpha =69.06^{\circ }}$. The particular values depend on the prism material, the wavelength of interest as well as on the compressor parameters.

Phase conjugation of chirped pulses

Chirped pulses from ${\displaystyle N}$ laser amplifiers may be phase locked via reflection from a phase-conjugating mirror^[7] to increase the brightness as ${\displaystyle N^{2}}$. For this purpose degenerate four-wave mixing Kerr Phase conjugation is relevant.^[8]

Other techniques

Some other techniques can be used for stretching and compressing pulses, but these are not suitable as the main stretcher/compressor in CPA due to their limited amount of dispersion and due to their inability to handle high-intensity pulses.

• A pulse can be stretched simply by letting it propagate through a thick slab of transparent material, such as 200 mm glass. As with the prisms, only a limited amount of dispersion can be achieved within physically practical dimensions. Outside the visible-light spectrum, materials exist both for positive and negative dispersion. For visible and near-infrared wavelengths, almost all transparent materials have positive dispersion. However, glass fibres can have their dispersion tailored to meet the needs.
• One or multiple reflections between a pair of chirped mirrors or similar device allow any form of chirp. This is often used in conjunction with the other techniques to correct for higher orders.
• The Dazzler is a commercial pulse shaper in which light is diffracted from an acoustic wave. By tuning the timing, frequency, and amplitude of the acoustic wave, it is possible to introduce arbitrary dispersion functions with a maximum delay of a few picoseconds.
• A phase-shifting mask can be placed in the focal plane of the stretcher in Fig. 3, which introduces additional dispersion. Such a mask can be an LCD array, where the phase shift can be tuned by changing the voltage on the pixels. This can generate arbitrary dispersion functions with a maximum of a few tens of picoseconds of delay. Such a setup is called a pulse shaper.

Applications

CPA is used in all of the highest-power lasers (greater than about 100 terawatts) in the world, with the exception of the ≈500 TW National Ignition Facility. Some examples of these lasers are the Vulcan laser at the Rutherford Appleton Laboratory's Central Laser Facility, the Diocles laser at the University of Nebraska–Lincoln, the GEKKO XII laser at the GEKKO XII facility in the Institute for Laser Engineering at Osaka University, the OMEGA and OMEGA EP lasers at the University of Rochester's Lab for Laser Energetics and the now dismantled petawatt line on the former Nova laser at the Lawrence Livermore National Laboratory. Gérard Mourou has proposed using CPA to generate high-energy and low-duration laser pulses to transmute highly radioactive material (contained in a target) to significantly reduce its half-life, from thousands of years to only a few minutes.^[9][10]

Apart from these state-of-the-art research systems, a number of commercial manufacturers sell Ti:sapphire-based CPAs with peak powers of 10 to 100 gigawatts.

See also

• Femtotechnology
• Group velocity
• Mode locking
• Raman amplification
• Regenerative amplification

References

1. Paschotta, Rüdiger (July 1, 2017). "Chirped-pulse Amplification". RP Photonics Encyclopedia. Retrieved October 2, 2018.
2. Strickland, Donna; Mourou, Gerard (1985). "Compression of amplified chirped optical pulses". Optics Communications. 56 (3). Elsevier BV: 219–221. Bibcode:1985OptCo..56..219S. CiteSeerX 10.1.1.673.148. doi:10.1016/0030-4018(85)90120-8. ISSN 0030-4018.
3. "The Nobel Prize in Physics 2018". Nobel Foundation. Retrieved 2 October 2018.
4. McCrory, Robert L. (October 2006). The Ultrafast Revolution of Chirped-Pulse Amplification from Tabletop Terawatts to Petawatt Laser Systems (PDF). Frontiers in Optics 2006. Rochester, NY.
5. Popmintchev, Dimitar; Wang, Siyang; Xiaoshi, Zhang; Stoev, Ventzislav; Popmintchev, Tenio (2022-10-24). "Analytical Lah-Laguerre optical formalism for perturbative chromatic dispersion". Optics Express. 30 (22): 40779–40808. Bibcode:2022OExpr..3040779P. doi:10.1364/OE.457139. PMID 36299007.
6. Popmintchev, Dimitar; Wang, Siyang; Xiaoshi, Zhang; Stoev, Ventzislav; Popmintchev, Tenio (2020-08-30). "Theory of the Chromatic Dispersion, Revisited". arXiv:2011.00066 [physics.optics].
7. Basov, N G; Zubarev, I G; Mironov, A B; Michailov, S I; Okulov, A Yu (1980). "Laser interferometer with wavefront reversing mirrors". Sov. Phys. JETP. 52 (5): 847. Bibcode:1980ZhETF..79.1678B.
8. Okulov, A Yu (2014). "Coherent chirped pulse laser network with Mickelson phase conjugator". Applied Optics. 53 (11): 2302–2311. arXiv:1311.6703. Bibcode:2014ApOpt..53.2302O. doi:10.1364/AO.53.002302. PMID 24787398. S2CID 118343729.
9. Fouquet, Helene; Root, Vidya N.; Warren, Hayley. "Nobel Prize Winner Could Have a Solution to Nuclear Waste". Bloomberg. Retrieved 2020-09-09.
10. "How Lasers Could Solve a Global Nuclear Waste Problem". April 8, 2019.