After Mary's death in 1857 Lyttelton married, secondly, Sybella Harriet Clive, daughter of George Clive MP, in 1869. They had three daughters:
The Honourable Sarah Kathleen Lyttelton (12 May 1870 – 1 October 1942); she married John Bailey on 26 April 1900. They had children.
The Honourable Sybil Lyttelton (17 February 1873 – 2 October 1934); she married Sir Lionel Cust on 16 July 1895. They had one son.
The Honourable Hester Margaret Lyttelton (26 December 1874 – 26 March 1958); she married Very Reverend Cyril Argentine Alington on 5 April 1904. They had six children.
Death
St John the Baptist Church, Hagley, grave of the 4th Baron Lyttelton and of his second wife Sybella Harriet (née Clive).St John the Baptist Church, Hagley, memorial to Sybella Harriet Lyttelton (née Clive, 1836–1900)St John the Baptist Church, Hagley, inscription inside the lychgate
In 1876 Lyttelton killed himself at the age of 59 by throwing himself down the stairs in a London house.[5] He was succeeded by his eldest son Charles, who later also inherited the viscounty of Cobham. Lady Lyttelton died in December 1900.
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