Samrat Chakrabarti is also an established international musician. In 1994, he founded Brandeis University's award-winning all male a cappella group, VoiceMale, for which he continues to contribute arrangements and original compositions, including "Please Don't Go," which appears on the album Suit Up and arrangements for the national a cappella compilation Voices Only 2009. He won a U.S. CARA for Best Original Pop/Rock Song for his composition "What's It all About". He is a former member of the a cappella group Five O' Clock Shadow. He was also a part of the group The Hyannis Sound. In 1998, Chakrabarti produced an untitled album for his musical group, JYDE, and composed the song "Startving".[citation needed]
Chakrabarti has also composed the theme song "Dhol Beat" for Loins of Punjab, and Sundaram Tagore's Natvar Bhavsar: Poetics of Color.[citation needed]