Pumpellyite crystallizes in the monoclinic-prismatic crystal system. It typically occurs as blue-green to olive green fibrous to lamellar masses. It is translucent and glassy with a Mohs hardness of 5.5 and a specific gravity of 3.2. It has refractive indices of nα=1.674–1.748, nβ=1.675–1.754 and nγ=1.688–1.764.
^Chesterman, Charles W. (1978). The Audubon Society field guide to North American rocks and minerals. New York: Alfred A. Knopf. p. 567. ISBN0394502698.